Povzetek

A series of fixed frequency dielectric measurements shows dielectric relaxation in La2CuMnO6, with a dynamic (Arrhenius to Arrhenius) crossover at TC. The external magnetic field alters the relaxation parameters in the vicinity of crossover and induces an unusual trend in the magnetodielectric coupling around TC. A large magnetodielectric coupling of 55% (at 68 K, 4 kHz) and 61% (at 105 K, 285.8 kHz) under a small magnetic field of 5 kOe is discovered. Presence of ferromagnetic short-range correlations above TC and a sign reversal of magnetoresistance around TC are observed. Specific heat analysis revealed the presence of ferromagnetic, variable range hopping active charge localized state. The presence of ferromagnetic short-range correlations and the influence of a core-grain dominated magnetoresistance on the Maxwell-Wagner interfacial polarization are responsible for the observed large magnetodielectric effect. Both the magnetic ordering and external magnetic field control the electric dipole relaxation in the material.

Ključne besede

double perovskite;griffiths-like phase;dielectric properties;magnetoresistance;magnetodielectric;

Podatki

Jezik: Angleški jezik
Leto izida:
Tipologija: 1.01 - Izvirni znanstveni članek
Organizacija: UNG - Univerza v Novi Gorici
UDK: 544
COBISS: 4979195 Povezava se bo odprla v novem oknu
ISSN: 0025-5408
Št. ogledov: 3093
Št. prenosov: 0
Ocena: 0 (0 glasov)
Metapodatki: JSON JSON-RDF JSON-LD TURTLE N-TRIPLES XML RDFA MICRODATA DC-XML DC-RDF RDF

Ostali podatki

URN: URN:SI:UNG
Vrsta dela (COBISS): Delo ni kategorizirano
Strani: str. 226-233
Zvezek: ǂVol. ǂ100
Čas izdaje: Apr. 2018
DOI: 10.1016/j.materresbull.2017.12.027
ID: 10892972