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Catalytic stereoconvergent synthesis of homochiral [beta]-CF[sub]3, [beta]-SCF[sub]3, and [beta]-OCF[sub]3 benzylic alcohols
Andrej Emanuel Cotman, Pavel A. Dub, Maša Sterle, Matic Lozinšek, Jaka Dernovšek, Živa Zajec, Anamarija Zega, Tihomir Tomašić, Dominique Cahard
Izvirni znanstveni članek
Oznake: adaptive crystals;asymmetric catalysis;density functional calculations;drug design;fluorine;hydrogenation;kinetic resolution;ruthenium;alcohols;catalysts;crystals;ketones;stereoselectivity;
We describe an efficient catalytic strategy for enantio- and diastereoselective synthesis of homochiral β-CF$_3$, β-SCF$_3$, and β-OCF$_3$ benzylic alcohols. The approach is based on dynamic kinetic resolution (DKR) with Noyori−Ikariya asymmetric transfer hydrogenation leading to simultaneous constr ...
Leto: 2022 Vir: Fakulteta za farmacijo (UL FFA)
Št. zadetkov: 1
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